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You won't find any itchy acrylic at this venerable Soho spot: Sisters and co-owners Joelle and Jennifer Hoverson fill their airy knitting-centric boutique with a kaleidoscope of vibrantly colored yarns spun from natural fibers such as silk, bamboo, alpaca and cashmere. You can also snap up crochet and felting kits as well as books on creating anything from afghans to bikinis.

Find more shops at Time Out New York.